Watervliet is a city in northeastern Albany County, New York, United States. The population was 10,375 as of the 2020 census. Watervlie…Watervliet is a city in northeastern Albany County, New York, United States. The population was 10,375 as of the 2020 census. Watervliet is north of Albany, the capital of the state, and is bordered on the north, west, and south by the town of Colonie. The city is also known as "the Arsenal City".
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